Spiroindoline derivatives having insecticidal properties 机翻标题: 暂无翻译,请尝试点击翻译按钮。

公开号/公开日
EP1694676 A1 2006-08-30 [EP1694676]EP1694676 B1 2009-08-26 [EP1694676] / 2006-08-302009-08-26
申请号/申请日
2004EP-0806344 / 2004-12-09
发明人
CASSAYRE JEROME;MOLLEYRES LOUIS-PIERRE;MAIENFISCH PETER;CEDERBAUM FREDRIK;
申请人
SYNGENTA PARTICIPATIONS;
主分类号
IPC分类号
A01N-043/40A01N-043/90A01N-047/38A61K-031/438C07D-471/10
摘要
(EP1694676) An insecticidal compound of formula (I), wherein Y is a single bond, C=O, C=S or S(O)m where m is 0, 1 or 2; R<1>, R<2>, R<3>, R<4>, R<8> A1, A2, A3, A4, B1, B2, B3 and B4 are specified organic groups or salts or N-oxides thereof; compositions containing them and their using in controlling insects, acarines, nematodes or molluscs.
机翻摘要
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地址
代理人
代理机构
;
优先权号
2003GB-0028908 2003-12-12 2004WO-IB04114 2004-12-09
主权利要求
(EP1694676)  1. A compound of formula I (see diagramm)wherein Y is a single bond, C=O, C=S or S(O) m where m is 0, 1 or 2; R **1 is hydrogen, optionally substituted alkyl, optionally substituted alkoxycarbonyl, optionally substituted alkylcarbonyl, aminocarbonyl, optionally substituted alkylaminocarbonyl, optionally substituted dialkylaminocarbonyl, optionally substituted aryl, optionally substituted heteroaryl, optionally substituted alkoxy, optionally substituted aryloxy, optionally substituted heteroaryloxy, optionally substituted heterocyclyloxy, cyano, optionally substituted alkenyl, optionally substituted alkynyl, optionally substituted cycloalkyl, optionally substituted cycloalkenyl, formyl, optionally substituted heterocyclyl, optionally substituted alkylthio, NO or NR **13R **14 where R **13 and R **14 are independently hydrogen, COR **15, optionally substituted alkyl, optionally substituted aryl, optionally substituted heteroaryl, optionally substituted heterocyclyl or R **13 and R **14 together with the N atom to which they are attached form a group -N=C(R **16)-NR **17R **18; R **15 is H, optionally substituted alkyl, optionally substituted alkoxy, optionally substituted aryl, optionally substituted aryloxy optionally substituted heteroaryl, optionally substituted heteroaryloxy or NR **19R **20; R **16, R **17 and R **18 are each independently H or lower alkyl; R **19 and R **20 are independently optionally substituted alkyl, optionally substituted aryl or optionally substituted heteroaryl; R **2 and R **3 are independently hydrogen, halogen, cyano, optionally substituted alkyl, optionally substituted alkoxy or optionally substituted aryl; each R **4 is independently halogen, nitro, cyano, optionally substituted C 1-8alkyl, optionally substituted C 2-6 alkenyl, optionally substituted C 2-6 alkynyl, optionally substituted alkoxycarbonyl, optionally substituted alkylcarbonyl, optionally substituted alkylaminocarbonyl, optionally substituted dialkylaminocarbonyl, optionally substituted C 3-7 cycloalkyl, optionally substituted aryl, optionally substituted heteroaryl, optionally substituted heterocyclyl, optionally substituted alkoxy, optionally substituted aryloxy, optionally substituted heteroaryloxy, optionally substituted alkylthio or R **21R **22N where R **21 and R **22 are, independently, hydrogen, C 1-8 alkyl, C 3-7 cycloalkyl, C 3-6 alkenyl, C 3-6 alkynyl, C 3-7 cycloalkyl(C 1- 4)alkyl, C 2-6haloalkyl, C 1-6 alkoxy(C 1-6)alkyl, C 1-6alkoxycarbonyl or R **21 and R **22 together with the N atom to which they are attached form a five, six or seven-membered heterocyclic ring which may contain one or two further heteroatoms selected from O, N or S and which may be optionally substituted by one or two C 1-6 alkyl groups, or 2 adjacent groups R **4 together with the carbon atoms to which they are attached form a 4, 5, 6,or 7 membered carbocyclic or heterocyclic ring which may be optionally substituted by halogen; n is 0,1, 2, 3 or 4; R **8 is optionally substituted alkyl, optionally substituted alkenyl, optionally substituted alkynyl, optionally substituted cycloalkyl, optionally substituted aryl, optionally substituted alkoxy, optionally substituted aryloxy, optionally substituted alkoxycarbonyl, optionally substituted alkylcarbonyl or optionally substituted alkenylcarbonyl; A 1, A 2, A 3, A 4, B 1, B 2, B 3 and B 4 are independently hydrogen, halogen, hydroxy, cyano, optionally substituted C 1-8 alkyl, optionally substituted C 2-6 alkenyl, optionally substituted C 2-6 alkynyl, optionally substituted alkoxycarbonyl, optionally substituted alkylcarbonyl, optionally substituted alkylaminocarbonyl, optionally substituted dialkylaminocarbonyl, optionally substituted C 3-7 cycloalkyl, optionally substituted aryl, optionally substituted heteroaryl, optionally substituted heterocyclyl, optionally substituted alkoxy, optionally substituted aryloxy, optionally substituted heteroaryloxy, optionally substituted alkylthio, optionally substituted arylthio or R **23R **24N where R **23 and R **24 are, independently, hydrogen, C 1-8 alkyl, C 3-7 cycloalkyl, C 3-6 alkenyl, C 3-6 alkynyl, C 3-7 cycloalkyl(C 1-4)alkyl, C 2-6 haloalkyl, C 1-6 alkoxy(C 1.  6)alkyl, C 1-6 alkoxycarbonyl or R **23 and R **24 together with the N atom to which they are attached form a five, six or seven-membered heterocyclic ring which may contain one or two further heteroatoms selected from O, N or S and which may be optionally substituted by one or two C 1-6 alkyl groups, or A 1 and A 2 together are =O, or A 3 and A 4 together are =O, or B 1 and B 2 together are =O, or B 3 and B 4 together are =O, or A 1 together with B 1 is a bond, or A 3 together with B 3 is a bond, or A 1 together with A 2 form with the carbon to which they are bound a three- to seven-membered ring, and may be saturated or unsaturated, and that may contain one or two hetero atoms selected from the group consisting of N, O and S, and which may be optionally substituted by one or two C 1-6 alkyl groups; or A 1 together with B 1 form with the carbon to which they are bound a three- to seven-membered ring, and may be saturated or unsaturated, and that may contain one or two hetero atoms selected from the group consisting of N, O and S, and which may be optionally substituted by one or two C 1-6 alkyl groups; or B 1 together with B 2 form with the carbon to which they are bound a three- to seven-membered ring, and may be saturated or unsaturated, and that may contain one or two hetero atoms selected from the group consisting of N, O and S, and which may be optionally substituted by one or two C 1-6 alkyl groups; or A 1 together with A 3 form a group -CH 2-, -CH=CH- or -CH 2CH 2; or B 1 together with B 3 form a group -CH 2-, -CH=CH- or -CH 2CH 2; or salts or N-oxides thereof provided that when B 1, B 2, B 3 and B 4 are all H, either both A 1 and A 2 are different from H or both A 3 and A 4 are different from H. 2. A compound according to claim 1 wherein Y is a single bond or C=O. 3. A compound according to claim 1 or claim 2 wherein R **2 and R **3 are each independently hydrogen, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or cyano. 4. A compound according to any preceeding claim wherein R **1 is hydrogen, C 1-6 alkyl, C 1-6 cyanoalkyl, C 1-6 haloalkyl, C 3-7 cycloalkyl(C 1-4)alkyl, C 1-6 alkoxy(C 1-6)alkyl, heteroaryl(C 1-6)alkyl (wherein the heteroaryl group may be optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy, C 1-6 haloalkoxy, C 1-6 alkylsulfonyl, C 1-6 alkylsulfinyl, C 1-6 alkylthio, C 1-6 alkoxycarbonyl, C 1-6 alkylcarbonylamino, arylcarbonyl, or two adjacent positions on the heteroaryl system may be cyclised to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring, itself optionally substituted with halogen), aryl(C 1-6)alkyl (wherein the aryl group may be optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy, C 1- 6 haloalkoxy, C 1-6 alkylsulfonyl, C 1-6 alkylsulfinyl, C 1-6 alkylthio, C 1-6 alkoxycarbonyl, C 1-6 alkylcarbonylamino, arylcarbonyl, or two adjacent positions on the aryl system may be cyclised to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring, itself optionally substituted with halogen), C 1-6 alkylcarbonylamino(C 1-6)alkyl, aryl (which may be optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy, C 1-6 haloalkoxy, C 1-6 alkylsulfonyl, C 1-6 alkylsulfinyl, C 1-6 alkylthio, C 1-6 alkoxycarbonyl, C 1-6 alkylcarbonylamino, arylcarbonyl, or two adjacent positions on the aryl system may be cyclised to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring, itself optionally substituted with halogen), heteroaryl (which may be optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy, C 1-6 haloalkoxy, C 1-6 alkylsulfonyl, C 1-6 alkylsulfinyl, C 1-6 alkylthio, C 1-6 alkoxycarbonyl, C 1-6 alkylcarbonylamino, arylcarbonyl, or two adjacent positions on the heteroaryl system may be cyclised to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring, itself optionally substituted with halogen), C 1-6 alkoxy, C 1-6 haloalkoxy, phenoxy (wherein the phenyl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), heteroaryloxy (optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), heterocyclyloxy (optionally substituted by halo, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), cyano, C 2-6 alkenyl, C 2-6 alkynyl, C 3-6 cycloalkyl, C 5-7 cycloalkenyl, heterocyclyl (optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), C 1-6 alkylthio, C 1-6 haloalkylthio or NR **13R **14 where R **13 and R **14 are independently hydrogen, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy(C 1-6)alkyl, phenyl (which may be optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino, dialkylamino or C 1-4 alkoxycarbonyl), phenyl (C 1-6)alkyl (wherein the phenyl group may be optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino, dialkylamino, C 1-6 alkylsulfonyl, C 1-6 alkoxycarbonyl, or two adjacent positions on the phenyl ring may be cyclised to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring, itself optionally substituted with halogen), heteroaryl (C 1-6)alkyl (wherein the heteroaryl group may be optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy, C 1-6 haloalkoxy, C 1-6 alkylsulfonyl, C 1-6 alkylsulfinyl, C 1-6 alkylthio, C 1-6 alkoxycarbonyl, C 1-6 alkylcarbonylamino, arylcarbonyl, or two adjacent positions on the heteroaryl system may be cyclised to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring, itself optionally substituted with halogen) or heteroaryl (which may be optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy, C 1-4 alkoxycarbonyl, C 1-6 alkylcarbonylamino, phenyloxycarbonylamino (wherein the phenyl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), amino, C 1-6 alkylamino or phenylamino (wherein the phenyl group is optionally substituted halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino)). 5. A compound according to any preceeding claim wherein each R **4 is independently halogen, cyano, C 1-8 alkyl, C 1-8 haloalkyl, C 1-6 cyanoalkyl, C 1-6 alkoxy(C 1-6)alkyl, C 3-7 cycloalkyl(C 1-6)alkyl, C 5-6 cycloalkenyl(C 1-6)alkyl, C 3- 6 alkenyloxy(C 1-6)alkyl, C 3-6 alkynyloxy(C 1-6)alkyl, aryloxy(C 1-6)alkyl, C 1-6 carboxyalkyl, C 1-6 alkylcarbonyl(C 1-6)alkyl, C 2-6 alkenylcarbonyl(C 1-6)alkyl, C 2-6 alkynylcarbonyl(C 1-6)-alkyl, C 1-6 alkoxycarbonyl(C 1-6)alkyl, C 3-6 alkenyloxycarbonyl(C 1-6)alkyl, C 3-6 alkynyloxycarbonyl(C 1-6)alkyl, aryloxycarbonyl(C 1-6)alkyl, C 1-6 alkylthio(C 1-6)alkyl, C 1-6 alkylsulfinyl(C 1-6)alkyl, C 1-6 alkylsulfonyl(C 1-6)alkyl, aminocarbonyl(C 1-6)alkyl, C 1-6alkylaminocarbony](C 1-6)alkyl, di(C 1-6)alkylaminocarbony](C 1-6)alkyl, pheny](C 1-4)alkyl (wherein the phenyl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), heteroaryl(C 1-4)alkyl (wherein the heteroaryl group is optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), heterocyclyi(C 1-4)alkyl (wherein the heterocyclyl group is optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), C 2-6 alkenyl, aminocarbonyl(C 2-6)alkenyl, C 1-6 alkylaminocarbonyl(C 2-6)alkenyl, di(C 1-6)alkylaminocarbonyl(C 2-6)alkenyl, phenyl(C 2-4)-alkenyl, (wherein the phenyl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), C 2-6 alkynyl, trimethylsilyl(C 2-6)alkynyl, aminocarbonyl(C 2-6)alkynyl, C 1-6 alkylaminocarbonyl(C 2-6)alkynyl, di(C 1-6)alkylaminocarbonyl(C 2-6)alkynyl, C 1-6 alkoxycarbonyl, C 3-7 cycloalkyl, C 3-7 halocycloalkyl, C 3-7 cyanocycloalkyl, C 1-3 alkyl(C 3-7)-cycloalkyl, C 1-3 alkyl(C 3-7)halocycloalkyl,phenyl (optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), heteroaryl (optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), heterocyclyl (wherein the heterocyclyl group is optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), or 2 adjacent groups R **4 together with the carbon atoms to which they are attached form a 4, 5, 6 or 7 membered carbocylic or heterocyclic ring which may be optionally substituted by halogen, C 1-8 alkoxy, C 1-6 haloalkoxy, phenoxy (optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), heteroaryloxy (optionally substituted by halo, nitro, cyano, C 1-6 alkyl, C 1-6 haloalkyl, C 1-6 alkoxy or C 1-6 haloalkoxy), C 1-8 alkylthio or R **19R **20N where R **19 and R **20 are, independently, hydrogen, C 1-8 alkyl, C 3-7 cycloalkyl, C 3-6 alkenyl, C 3-6 alkynyl, C 2-6 haloalkyl, C 1-6 alkoxycarbonyl or R **19 and R **20 together with the N atom to which they are attached form a five, six or seven-membered heterocyclic ring which may contain one or two further heteroatoms selected from O, N or S and which may be optionally substituted by one or two C 1-6 alkyl groups; and n is 0, 1, 2 or 3. 6. A compound according to any preceeding claim wherein R **8 is C 1-10 alkyl, C 1-10 haloalkyl, aryl(C 1-6)alkyl (wherein the aryl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), heteroaryl (C 1-6)alkyl (wherein the heteroaryl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), arylcarbonyl-(C 1-6)alkyl (wherein the aryl group may be optionally substituted by halogen, C 1-4alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino and the alkyl group may be optionally substituted by aryl), C 2-8 alkenyl, C 2-8 haloalkenyl, aryl(C 2-6)-alkenyl (wherein the aryl group is optionally substituted halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino, C 1-6 alkoxycarbonyl, or two adjacent substituents can cyclise to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring), heteroaryl(C 2-6)-alkenyl (wherein the heteroaryl group is optionally substituted halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino, C 1-6 alkoxycarbonyl, or two adjacent substituents can cyclise to form a 5, 6 or 7 membered carbocyclic or heterocyclic ring), C 2-6 alkynyl, phenyl(C 2-6)alkynyl (wherein the phenyl group is optionally substituted by halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4 haloalkoxy, CN, NO 2, aryl, heteroaryl, amino or dialkylamino), C 3-7 cycloalkyl, C 1-6 alkoxycarbonyl, C 1-6 alkylcarbonyl, C 1-6 haloalkylcarbonyl or aryl(C 2-6)alkenylcarbonyl (wherein the aryl group may be optionally substituted halogen, C 1-4 alkyl, C 1-4 alkoxy, C 1-4 haloalkyl, C 1-4haloalkoxy, CN, NO 2 aryl, heteroaryl, amino or dialkylamino), or -C(R **51)(R **52)-[CR **53=CR **54]z-R **55 where z is 1 or 2, R **51 and R **52 are each independently H, halo or C 1-2alkyl, R **53 and R **54 are each independently H, halogen, C 1-4 alkyl or C 1-4 haloalkyl and R **55 is optionally substituted aryl or optionally substituted heteroaryl. 7. A compound according to any preceeding claim wherein A 1, A 2, A 3, A 4, B 1, B 2, B 3 and B 4 are independently each hydrogen, halo, cyano, C 1-3 alkyl, hydroxy or two groups attached to the same carbon atom together with the carbon atom form a carbonyl group. 8. A compound of formula (II) (see diagramm) wherein Y, n, R **1, R **2, R **3, R **4, A 1, A 2, A 3, A 4, B 1, B 2, B 3 and B 4 are as defined in claim 1 and R **8 is hydrogen or tert-butoxycarbonyl. 9. An insecticidal, acaricidal or nematicidal composition comprising an insecticidally, acaricidally or nematicidally effective amount of a compound of formula I as defined in claim 1. 10. A method of combating and controlling insects, acarines, nematodes or molluscs which comprises applying to a pest, to a locus of a pest, or to a plant susceptible to attack by a pest an insecticidally, acaricidally, nematicidally or molluscicidally effective amount of a compound of formula I, provided the method is not for the treatment of the human or animal body by therapy.
法律状态
(EP1694676) LEGAL DETAILS FOR EP1694676  Actual or expected expiration date=2016-01-29    Legal state=DEAD    Status=LAPSED     Event publication date=2004-12-09  Event code=EP/APP  Event indicator=Pos  Event type=Examination events  Application details  Application country=EP EP04806344  Application date=2004-12-09  Standardized application number=2004EP-0806344     Event publication date=2006-08-30  Event code=EP/A1  Event type=Examination events  Application published with search report  Publication country=EP  Publication number=EP1694676  Publication stage Code=A1  Publication date=2006-08-30  Standardized publication number=EP1694676     Event publication date=2006-08-30  Event code=EP/AK  Event indicator=Pos  Event type=Designated states  Designated contracting states: Benannte vertragsstaaten AT BE BG CH CY CZ DE DK EE ES FI FR GB GR HU IE IS IT LI LT LU MC NL PL PT RO SE SI SK TR    Event publication date=2006-08-30  Event code=EP/17P  Event indicator=Pos  Event 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state=CZ     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=CZ   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR DE602004022854  Actual or expected expiration date=2015-07-01    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=DE Corresponding appl: DE602004022854  Application date in the designated or member state=2004-12-09   Application number in the designated or member state=2004DE-60022854 Corresponding cc:  Designated or member state=DE Corresponding pat: DE602004022854  Publication stage code in the designated or member state=D1  Publication date in the 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verfallen Corresponding cc:  Designated or member state=DE     Event publication date=2015-07-01  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=DE   Effective date of the event=2015-07-01  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR DK  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=DK     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=DK   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR EE  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=EE     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=EE   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR ES2332723  Actual or expected expiration date=2016-01-29    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=ES Corresponding appl: ES04806344  Application date in the designated or member state=2004-12-09   Application number in the designated or member state=2004ES-0806344T Corresponding cc:  Designated or member state=ES Corresponding pat: ES2332723  Publication stage code in the designated or member state=T3  Publication date in the designated or member state=2010-02-11   Publication number in the designated or member state=ES2332723    Event publication date=2010-02-11  Event code=EP/REG  Event code=ES/FG2A  Event indicator=Pos  Event type=Event indicating In Force  Reference to a national code Definitive protection Proteccion definitiva Corresponding cc:  Designated or member state=ES     Event publication date=2013-12-17  Event code=EP/PGFP  Event indicator=Pos  Event type=Event indicating In Force  Event type=Payment or non-payment notifications  Postgrant: annual fees paid to national office   Annual fees payment date=2013-12-17     Year of payment of annual fees=10  Corresponding cc:  Designated or member state=ES     Event publication date=2014-12-10  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=ES   Effective date of the event=2014-12-10  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES     Event publication date=2016-01-29  Event code=EP/REG  Event code=ES/FD2A  Event indicator=Neg  Event type=Event indicating Not In Force  Reference to a national code Announcement of lapse in spain Ep-patente caducidades Corresponding cc:  Designated or member state=ES   Effective date of the event=2016-01-29  MEMBER STATE LEGAL DETAILS FOR FI  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=FI     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a 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code=EP/PGFP  Event indicator=Pos  Event type=Event indicating In Force  Event type=Payment or non-payment notifications  Postgrant: annual fees paid to national office   Annual fees payment date=2013-11-26     Year of payment of annual fees=10  Corresponding cc:  Designated or member state=GB     Event publication date=2014-12-09  Event code=EP/GBPC  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  GB: European patent ceased through non-payment of renewal fee Corresponding cc:  Designated or member state=GB   Effective date of the event=2014-12-09     Event publication date=2014-12-09  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=GB   Effective date of the event=2014-12-09  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR GR  Actual or expected expiration date=2009-11-27    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=GR     Event publication date=2009-11-27  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=GR   Effective date of the event=2009-11-27  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR HU  Actual or expected expiration date=2010-02-27    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=HU     Event publication date=2010-02-27  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=HU   Effective date of the event=2010-02-27  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR IE  Actual or expected expiration date=2009-12-09    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=IE     Event publication date=2009-09-30  Event code=EP/REG  Event code=IE/FG4D  Event indicator=Pos  Event type=Event indicating In Force  Reference to a national code European patents granted designating ireland Corresponding cc:  Designated or member state=IE     Event publication date=2009-12-09  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=IE   Effective date of the event=2009-12-09  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR IS  Actual or expected expiration date=2009-12-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=IS     Event publication date=2009-12-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=IS   Effective date of the event=2009-12-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR IT  Actual or expected expiration date=2014-12-09    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=IT     Event publication date=2013-12-18  Event code=EP/PGFP  Event indicator=Pos  Event type=Event indicating In Force  Event type=Payment or non-payment notifications  Postgrant: annual fees paid to national office   Annual fees payment date=2013-12-18     Year of payment of annual fees=10  Corresponding cc:  Designated or member state=IT     Event publication date=2014-12-09  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=IT   Effective date of the event=2014-12-09  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR LI  Actual or expected expiration date=2009-12-31    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=LI     Event publication date=2009-12-31  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=LI   Effective date of the event=2009-12-31  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR LT  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=LT     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=LT   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT     Event publication date=2010-01-25  Event code=EP/LTIE  Event indicator=Neg  Event type=Event indicating Not In Force  LT: Invalidation of european patent or patent extension LT: Invalidation of european patent extension Corresponding cc:  Designated or member state=LT   Effective date of the event=2009-08-26  MEMBER STATE LEGAL DETAILS FOR LU  Actual or expected expiration date=2009-12-09    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=LU     Event publication date=2009-12-09  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=LU   Effective date of the event=2009-12-09  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR MC  Actual or expected expiration date=2010-07-01    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=MC     Event publication date=2010-07-01  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=MC   Effective date of the event=2010-07-01  LAPSE BECAUSE OF NON-PAYMENT OF DUE FEES  MEMBER STATE LEGAL DETAILS FOR NL  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=NL     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=NL   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT     Event publication date=2010-02-01  Event code=EP/NLV1  Event indicator=Neg  Event type=Event indicating Not In Force  NL: Lapsed or annuled due to failure to fulfill the requirements of Art. 29p and 29m of the patents act  no legal effect from NL: wirkung in nl nicht eingetreten (Art. 29p und 29m nl patg.) Corresponding cc:  Designated or member state=NL  MEMBER STATE LEGAL DETAILS FOR PL  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=PL     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=PL   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR PT  Actual or expected expiration date=2009-12-28    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=PT     Event publication date=2009-12-28  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=PT   Effective date of the event=2009-12-28  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR RO  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=RO     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=RO   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR SE  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=SE     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=SE   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR SI  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=SI     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=SI   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR SK  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=SK     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=SK   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT  MEMBER STATE LEGAL DETAILS FOR TR  Actual or expected expiration date=2009-08-26    Legal state=DEAD    Status=LAPSED   Corresponding cc:  Designated or member state=TR     Event publication date=2009-08-26  Event code=EP/PG25  Event indicator=Neg  Event type=Event indicating Not In Force  Event type=Payment or non-payment notifications  Lapsed in a contracting state announced via postgrant inform. from nat. office to EPO Corresponding cc:  Designated or member state=TR   Effective date of the event=2009-08-26  LAPSE BECAUSE OF FAILURE TO SUBMIT A TRANSLATION OF THE DESCRIPTION OR TO PAY THE FEE WITHIN THE PRESCRIBED TIME-LIMIT
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